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In the experimental setup, volcanic ash was suspended in nitrogen through mechanical agitation. Extinction spectra were recorded in the infrared, visible, and ultraviolet spectral regions. The particle size distribution within the airflow was also recorded. An iterative algorithm allowed us to obtain fully consistent CRIs for the six samples, compatible with the observed extinction spectra and the Kramers-Krönig relations. While a good agreement is found with other recently reported CRIs in the UV/Vis, larger differences are found in the