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Additionally, the UiO-66-NMe3+ could be well regenerated by simple solvent washing and exhibited a slight decline of adsorption capacity after seven successive recycle. Furthermore, satisfactory adsorption capacity and reusability of the MOFs in environmental water samples were attained. Comparing with reported activated carbon and resin materials, the UiO-66-NMe3+ MOFs possessed higher adsorption capacity and shorter equilibrium time, as well as good reusability and practicality. The developed ion-exchange functionalized MOFs provided