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echanisms that govern the electroactive membrane technology. Then we summarize our findings on the rational design of several flow-through electrochemical CNT filtration systems focused on either anodic oxidation reactions or cathodic reduction reactions. Subsequently, we discuss a recently discovered electrochemical valence-state-regulation strategy that is capable to detoxify and sequester heavy metal ions. Finally, we conclude the Account with our perspectives toward future development of the electroactive membrane technology.Passiva