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In this work, such heterogeneous damage was further conquer in NixFe1-x solitary crystal alloys via a simple method of fine-tuning the structure. [001] NixFe1-x (x = 0, 0.38 and 0.62 at%) single crystals prepared making use of the Bridgman strategy were irradiated over a wide fluence range (4 × 1013 to 4 × 1015 ions per cm2). The irradiation-induced defect advancement ended up being studied utilizing Rutherford backscattering/channeling spectrometry, Monte Carlo simulati