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Therefore, it is essential to know the way the construction of spacer ligands influences the direction and phase distribution of resulting 2D perovskite films. In this work, a brand new member of Dion-Jacobson (DJ) phase 2D perovskites based on trans-1,4-cyclohexanediamine (CHDA) is shown which is discovered that the crystalline orientation is self-aligned spontaneously, that is distinct from the popular graded distribution in controlled test along
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