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The most active catalyst R-Cryptomelane reached a current density of 10 mA cm -2 at a potential 1.73 V without, and at 1.71 V in presence of carbon black. The improvement was significantly higher for catalyst with lower initial activity. However, the materials showed a disappointing catalytic stability during alkaline electrochemical OER, while the crystal structure was found to be stable at working conditions. © 2020 WILEY-VCH Verlag GmbH Co. KGaA, Weinheim.To design high-performance mid-infrared (IR) nonlinear optical (NLO) mate
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