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Surface chemistry and photochemistry of small molecules on the rutile TiO2(001) and TiO2(011)-(2 × 1) surfaces were studied by low energy electron diffraction, thermal desorption spectroscopy, and x-ray photoelectron spectroscopy. It was found that the TiO2(001) surface mainly exhibits the defects of Ti interstitials in the near-surface region, while the TiO2(011)-(2 × 1) surface mainly exhibits the defects of double-oxygen vacancies. The defect structures of TiO2 surfaces strongly affect their adsorption and thermal/photodesorption beha
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