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Previous publications have demonstrated the tuning of ion-transfer (IT) processes across ion-selective membranes (ISMs) with thicknesses in the nanometer order by modulating the oxidation state of a film of a conducting polymer, such as poly(3-octylthiophene) [POT], that is in back-side contact. Attempts on the theoretical description of this charge transfer (CT)-IT system have considered the Nernst equation for the CT, while there is no empirical evidence confirming this behavior. We present herein the first experimental characterization
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