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Developing efficient photocatalysts for synchronously producing H2 and high value-added chemicals holds great promise to enhance solar energy conversion. Herein, a facile strategy of simultaneously engineering Pd cocatalyst and oxygen vacancies (VO s) on TiO2 to promote H2 production coupled with selective oxidation of benzylamine is demonstrated. The optimized PdSA+C /TiO2 -VO photocatalyst containing Pd single atoms (SAs), clusters (C), and VO s exhibits much superior performance to those of TiO2 -VO and PdSA /TiO2 -VO counterparts.
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