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Flexible pressure sensors with high sensitivity over a broad pressure range are highly desired, yet challenging to build to meet the requirements of practical applications in daily activities and more significant in some extreme environments. This work demonstrates a thin, lightweight, and high-performance pressure sensor based on flexible porous phenyl-silicone/functionalized carbon nanotube (PS/FCNT) film. The formed crack-across-pore endows the pressure sensor with high sensitivity of 19.77 kPa-1 and 1.6 kPa-1 in the linear range of