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Overall, our findings provide a good illustration of the need to use short-wavelength VUV probes to obtain the most comprehensive picture possible in photoionization-based studies of photochemical dynamics.A strategy to create organic molecules with high degrees of radical spin multiplicity is reported in which molecular design is correlated with the behaviour of radical anions in a series of BODIPY dyads. Upon reduction of each BODIPY moiety radical anions are formed which are shown to have different spin multiplicities by electron par
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