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Modification of chitosan material introducing long-distanced amino groups significantly influences the intramolecular interactions within a single polymer chain, thus blocking the access of diclofenac to the biopolymer backbone. The strongest attraction between two chitosan chains with two long-distanced amino groups can exceed 120 kcal/mol, while the modified chitosandiclofenac interaction remains of the order of 20 to 40 kcal/mol. Background Genista tridentata L. is an endemic species from the Iberian Peninsula used in Portuguese tra