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The deviations observed in the fragility-DS/DV relationship are shown to be correlated to the extent of segregation or depletion of the mobile element at the surface. Finally, we explore the relationship between the diffusion pre-exponential factor (D and the activation energy (Q) and compare it to a ln(D-Q correlation previously established for bulk glasses, demonstrating similar correlations from MD as in the experiments and that the surface and bulk have very similar ln(D-Q correlations.Computational schemes for comprehensive stu
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