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The neat and aqueous solutions of the cholinium glycinate ionic liquid (IL), [Cho][Gly], at different water mole fractions, xws, are studied by molecular dynamics simulations. The changes in the local nanostructure of systems with composition have been determined by calculation of various structural distribution functions. Hydrogen bond (H-bond) attractions determine the major relative orientations of the oppositely and like charged nearest neighbors. The cation-anion H-bonds mainly form between the hydrogen of the hydroxyl or methyl gr
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