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Transparent photovoltaics are receiving increased attention for their wide range of applicability, but there have been few attempts to systematically tune organic materials to achieve transparency. In this Letter, we study the influence of simple structural modifications on the photoabsorption spectrum of the nonfullerene electron acceptor perylenediimide. Motivated by push-pull design strategies, we explore the effects of applying electron-donating functional groups with varying strengths using three design motifs. We demonstrate that
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