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The obtained numerical and experimental results showed that the metamaterial with rainbow blocks has extended bandgaps compared with the periodic metamaterial.The traditional methods for preparing magnesium aluminum layered double hydrotalcite (Mg2Al-CO3LDHs) in industry include coprecipitation and hydrothermal methods. Both these methods have the disadvantages of high preparation cost and complicated water washing process. Using Mg(OH)2, Al(OH)3, and CO2 as raw materials in this work, the Mg2Al-CO3 LDHs are successfully prepared by mech