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This work not only contributes to long-term stable operation of high-voltage LIBs but also brings new opportunities for the development of next-generation 5 V LIBs.Soft robotics focuses on mimicking natural systems to produce dexterous motion. Dielectric elastomer actuators (DEAs) are an attractive option due to their large strains, high efficiencies, lightweight design, and integrability, but require high electric fields. Conventional approaches to improve DEA performance by incorporating solid fillers in the polymer matrices can incr