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Inspection of the aggregate morphology shows that the formed clusters are composed of few minority particles placed in the inner region, while the aggregate surface is covered by majority particles, acting to provide a shielding effect against further growth.The crystal quality of a Cu2ZnSn(S,Se)4 (CZTSSe) thin film is crucially important to a high-performance CZTSSe solar cell. After selenization, a bilayer CZTSSe thin film consisting of a large-grain top layer and a small-particle bottom layer is usually observed according to the litera
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