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Particularly, the visible-light activity is enhanced by 10 times by using Au. Incorporating the experimental outcome plus the theoretic calculation, both of hydrogen treatment and Au loading help form nitrogen vacancies on carbon nitride nanosheets, which advertise N 2 activation by enhancing the chemisorption. Meanwhile, the Au running further improves the nitrogen decrease performance through billing the excited hot electrons created through the area plasmonic resonance into the adsorbed N 2 mol