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The Ca1-xCrxO systems have actually correct half-metallicities, which are verified by the spin polarization of 100% plus the integer values of complete magnetic moments. The Ca0.75Cr0.25O, Ca0.5Cr0.5O, and Ca0.25Cr0.75O tend to be half-metallic ferromagnetic with flip-gaps of 1.495, 0.888, and 0.218 eV, correspondingly. Therefore, the Ca1-xCrxO materials are ideal applicants for possible applications of spin-injection in future semiconductors spintronics.A binary hybrid system c