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0001] and PM10 [slope = 0.46 (±0.09); p-value less then 0.0001] samples. Measurements at the Harvard Supersite and at EPA RadNet sites are highly correlated for both α-activities [slope = 0.17 (±0.02), p-value less then 0.0001] and β-activities [slope = 0.30 (±0.05), p-value less then 0.0001]. Additionally, we identified several significant predictors for PM2.5 α-activities. This novel method we developed to measure α- and β-activities from archived filters will make it possible to assess the retrospective particle radioactivity exposure