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The Cd content in the soil is extremely negatively correlated with the BCF of wheat, summer maize, and spring maize. The relationship between soil organic matter (SOM) and the BCF of wheat and summer maize demonstrated a significant negative correlation. The soil pH and cation exchange capacity (CEC) also affect the BCF of crops. Introducing the soil Cd content, pH, SOM, CEC, and other factors, the Cd bioaccumulation factor prediction equations of rice, wheat, summer maize, and spring maize were established. The correlation coefficients