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Soil enzyme activities including dehydrogenase, urease, and catalase increased up to 5-fold. Soil bacterial diversity and structure were changed, being largely composed of Proteobacteria, Actinobacteria, Patescibacteria, Bacteroidetes, and Firmicutes. These findings provide a green and sustainable approach to decontaminating complex-polluted environments with comprehensive improvement of soil health.The nanoparticles of zeolitic imidazolate framework (ZIF-67) were synthesized and added to ethanolamine/deep eutectic solvent solution to f