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Nanocelluloses, both cellulose nanofibrils and cellulose nanocrystals, are gaining research traction due to their viability as key components in commercial applications and industrial processes. Significant efforts have been made to understand both the potential of assembling nanocelluloses, and the limits and prospectives of the resulting structures. This Review focuses on bottom-up techniques used to prepare nanocellulose-only structures, and details the intermolecular and surface forces driving their assembly. Additionally, the interac
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