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The synthesis and diverse changes of a dinitrogen dititanium hydride complex bearing the rigid acridane-based acri PNP-pincer ligands are presented. This complex enabled N2 cleavage and hydrogenation also without extra H2 or any other reducing agents. Furthermore, diverse changes regarding the N2 unit with many different organometallic compounds such as for example ZnMe2 , MgMe2 , AlMe3 , B(C6 F5 )3 , PinBH, and PhSiH3 being more successful at the rigid acri PNP-ligated dititanium fram
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