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A finite chain of thirty-one paramagnetic centers is reported, synthesized by reaction of hydrated chromium fluoride, copper carbonate and pivalic acid in the presence of 1,4,7,10-tetrazacyclododecane (cyclen). Magnetic studies show predominantly anti-ferromagnetic exchange leading to a high density of low-lying spin states and large saturation field.First-principles simulations can advance our understanding of phase transitions but are often too costly for the heavier elements, which require a relativistic treatment. Addressing this cha
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