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Halide perovskite (HP) single crystals (SCs) are garnering extensive attention as active materials to substitute polycrystalline counterparts in solar cells, photodiodes, and photodetectors, etc. Nevertheless, the large thickness and defect-rich surface results in severe carrier recombination and becomes the major bottleneck for augmented performance. In this perspective, we are looking forward to explaining in detail why the SCs hardly unleash their engrossing potential and introduce two parallel paths for further advancement. First is