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This paper presents a sparse spectral unmixing algorithm for activity estimation of radionuclides in γ-ray spectrometry. The spectral unmixing method aims to decompose a measured spectrum into spectral signatures of radionuclides, which is sensitive to the choice of the spectral signatures. The sparsity of the solution is imposed to identify the active radionuclides. Experimental results on simulated and real spectra show that the proposed method yields significant improvement for estimating radioactivity at low statistics. Automated produ

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