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Herein, edge-rich straight graphene (er-VG) was synthesized and utilized as a catalyst assistance for Ni-Fe hydroxides when it comes to air evolution effect (OER). The hybrid Ni-Fe/er-VG catalyst displays exceptional OER overall performance with a mass current of 4051 A g-1 (at overpotential η = 300 mV) and return frequency (TOF) of 4.8 s-1 (η = 400 mV), outperforming Ni-Fe deposited on pristine VG as well as other steel foam supports. Angle-dependent X-ray absorption spectroscopy demonstrates the

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