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One of the encouraging processes to protect the environment is the catalytic conversion of N2O and other harmful greenhouse gases. Employing heteroatom dopants into the Graphene structure for this conversion is an attractive technique owing to its relatively low price and the very low destructive impacts. DFT was applied to explore fundamental and principal reactions of N2O adsorption and dissociation over the Silicon-embedded Graphene catalyst to contribute to the search for green catalysts in the conversion of toxic gases into less h