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All rights reserved.Modification of this outside areas of metal organic frameworks offers a unique amount of control of their particular adsorption behavior. We have formerly shown that capping of MOFs with ethylenediamine (EDA) can successfully keep small gaseous molecules [Nat. Comm. 2016, 7, 13871] at room temperature . Here, we report a temperature-induced difference into the capping-layer gate opening process through a variety of in situ IR experiments and ab initio simulations regarding the
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