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Herein we report how an anode is eroded and the eroded mass is deposited on the cathode surface at different arc currents ([Formula see text]) in a DC carbon arc discharge using roughly oriented graphite (ROG) as electrodes. It was found that the nature of anode erosion critically depends on [Formula see text] and has profound effects on the morphology of the as-synthesized cathode deposits (CDs), the conversion efficiency of the system to form the CDs and their compositions. By characterizing the as-synthesized CDs in their totality b
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