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The emission ratios of five pollutants were simultaneously adjusted during the RSM-assimilation, indicating that the emission inventory may underestimate NO2 in January, April and October, and SO2 in April, but overestimate NH3 in April and VOC in January and October. Primary PM2.5 emissions are also significantly underestimated, particularly in April (dust season in NCP). Future work should focus on expanding the control area and including NH3 observations to improve the RSM-assimilation performance and emission inventories.Traditional watershed modeling o