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Our results provide important insights into the structural origin of the emergent anisotropic and cooperative heterogeneous dynamics, and we discuss analogies with previous work on other soft disordered systems.Amide naphthotubes with four carboxylate sidechains have been reported by us for selectively recognizing hydrophilic molecules in water and they have found applications in sensing and self-assembly. Modification of these macrocycles on the sidechains would further expand their applicability. Herein, we report the synthesis of mono-functionalized amid
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