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with transient absorption spectroscopy from the UV continuously into the mid-infrared, along with time-resolved Raman and emission and magnetic resonance spectroscopies to build a complete and detailed molecular level picture of the dynamics of these dimers. The knowledge gained from dimer studies can also be applied to the understanding the dynamics in extended molecular solids. The insight afforded by these studies will help guide the creation of new designer chromophores with control over the fate of the excited state.Electromagnetic