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Our device is highly promising in the applications of thermo-tunable modulators and obtaining single frequency near-infrared signals from broadband sources.We report on continuous-wave laser operation of Tb3+LiLuF4 under UV pumping. More than five times higher absorption cross sections in the UV allow for shorter gain media, which are required for future high-power diode pumping. The cross-relaxation process is found to efficiently populate the upper laser level 5D4 at doping concentrations typically used in Tb3+-doped gain media. Pumpi
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